2024
Simulating Chemistry on Bosonic Quantum Devices
Dutta R, Cabral D, Lyu N, Vu N, Wang Y, Allen B, Dan X, Cortiñas R, Khazaei P, Schäfer M, Albornoz A, Smart S, Nie S, Devoret M, Mazziotti D, Narang P, Wang C, Whitfield J, Wilson A, Hendrickson H, Lidar D, Pérez-Bernal F, Santos L, Kais S, Geva E, Batista V. Simulating Chemistry on Bosonic Quantum Devices. Journal Of Chemical Theory And Computation 2024, 20: 6426-6441. PMID: 39068594, DOI: 10.1021/acs.jctc.4c00544.Peer-Reviewed Original ResearchQuantum devicesQuantum two-level systemTwo-level systemMolecular vibronic spectraCalculations of electronic structureQuantum simulationBoson operatorsSystem HamiltonianQuantum computationVibronic spectraElectronic structureChemical dynamicsSolution-phaseReview recent progressGas-phaseChemical structureChemical problemsRecent progressCalculationsSimulate chemistryBosonsHamiltonianOscillationsDynamicsDevices
2020
Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor
Wang C, Curtis J, Lester B, Zhang Y, Gao Y, Freeze J, Batista V, Vaccaro P, Chuang I, Frunzio L, Jiang L, Girvin S, Schoelkopf R. Efficient Multiphoton Sampling of Molecular Vibronic Spectra on a Superconducting Bosonic Processor. Physical Review X 2020, 10: 021060. DOI: 10.1103/physrevx.10.021060.Peer-Reviewed Original ResearchMolecular vibronic spectraMultiphoton quantum statesVibronic spectraLinear optical systemsVibrational excited statesOptical photonsKerr interactionPhoton numberQuantum statesSuperconducting architecturesQuantum systemsOptical systemExcited statesQuantum machineBosonic systemsSuperconducting devicesGaussian operationsPhotoelectron processesInput statesMolecular ensemblesBosonic structurePhotonsPromising platformSpectraEfficient preparation