2025
Photoelectrocatalytic reduction of CO2 to formate using immobilized molecular manganese catalysts on oxidized porous silicon
Hong Y, Jia X, Stewart-Jones E, Kumar A, Wedal J, Alvarez-Hernandez J, Donley C, Gang A, Gibson N, Hazari N, Houck M, Jeon S, Kim J, Koh H, Mayer J, Mercado B, Nedzbala H, Piekut N, Quist C, Stach E, Zhang Y. Photoelectrocatalytic reduction of CO2 to formate using immobilized molecular manganese catalysts on oxidized porous silicon. Chem 2025, 11: 102462. PMID: 40894117, PMCID: PMC12396503, DOI: 10.1016/j.chempr.2025.102462.Peer-Reviewed Original ResearchCO2 reduction to formateReduction to formateMolecular catalystsManganese complexesReduction of CO2 to formateReduction of carbon dioxideCO2 to formatePorous siliconBpy ligandsHybrid photoelectrodesManganese catalystsSilatrane groupSun illuminationCO2 reductionCatalystExcellent reproducibilitySemiconducting siliconCurrent densityPorous silicon waferOxidized porous siliconPhotoelectrodeManganeseSilatranesCarbon dioxidePhotoelectrocatalysts
2024
Room‐Temperature Formate Ester Transfer Hydrogenation Enables an Electrochemical/Thermal Organometallic Cascade for Methanol Synthesis from CO2
Fernández S, Assaf E, Ahmad S, Travis B, Curley J, Hazari N, Ertem M, Miller A. Room‐Temperature Formate Ester Transfer Hydrogenation Enables an Electrochemical/Thermal Organometallic Cascade for Methanol Synthesis from CO2. Angewandte Chemie International Edition 2024, 64: e202416061. PMID: 39571086, DOI: 10.1002/anie.202416061.Peer-Reviewed Original ResearchTransfer hydrogenationMethanol synthesisIsopropyl formateReduction of CO2 to methanolCO2 reduction to formateCO2 to methanolHydrogen bonding interactionsReduction to formateFormate to methanolEnergy-dense liquid fuelsRoom temperature reductionMulticatalyst systemsOrganometallic catalystsOrganometallic reactionsFormate ionTrifluoromethanesulfonic acidBonding interactionsFischer esterificationFormate estersIsopropanol solventHydrogenMethanolEster substratesElectrocatalystsEnergy storageRoom‐Temperature Formate Ester Transfer Hydrogenation Enables an Electrochemical/Thermal Organometallic Cascade for Methanol Synthesis from CO2
Fernández S, Assaf E, Ahmad S, Travis B, Curley J, Hazari N, Ertem M, Miller A. Room‐Temperature Formate Ester Transfer Hydrogenation Enables an Electrochemical/Thermal Organometallic Cascade for Methanol Synthesis from CO2. Angewandte Chemie 2024, 137 DOI: 10.1002/ange.202416061.Peer-Reviewed Original ResearchTransfer hydrogenationMethanol synthesisIsopropyl formateReduction of CO2 to methanolCO2 reduction to formateCO2 to methanolHydrogen bonding interactionsReduction to formateFormate to methanolEnergy-dense liquid fuelsRoom temperature reductionMulticatalyst systemsOrganometallic catalystsOrganometallic reactionsFormate ionTrifluoromethanesulfonic acidBonding interactionsFischer esterificationFormate estersIsopropanol solventHydrogenMethanolEster substratesElectrocatalystsEnergy storage
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