Tailoring Interfaces for Enhanced Methanol Production from Photoelectrochemical CO2 Reduction
Shang B, Zhao F, Suo S, Gao Y, Sheehan C, Jeon S, Li J, Rooney C, Leitner O, Xiao L, Fan H, Elimelech M, Wang L, Meyer G, Stach E, Mallouk T, Lian T, Wang H. Tailoring Interfaces for Enhanced Methanol Production from Photoelectrochemical CO2 Reduction. Journal Of The American Chemical Society 2024, 146: 2267-2274. PMID: 38207288, DOI: 10.1021/jacs.3c13540.Peer-Reviewed Original ResearchFaradaic efficiencyReduction of CO<sub>2</sub>Conversion of CO<sub>2</sub>Accumulation of reaction intermediatesParasitic side reactionsPartial current densityOne-electron reductionCO2 reduction efficiencyEnhanced methanol productionCurrent densityElectrode surface areaThermodynamic driving forceMolecular catalystsPhotoelectrochemical conversionCatalyst loadingCatalyst surfaceSilicon photoelectrodesReaction intermediatesSide reactionsMicropillar array structureLight absorptionCarbon layerGaseous intermediatesSurface areaMethanol production
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