Tuning the Protein‐Induced Absorption Shifts of Retinal in Engineered Rhodopsin Mimics
Suomivuori C, Lang L, Sundholm D, Gamiz‐Hernandez A, Kaila V. Tuning the Protein‐Induced Absorption Shifts of Retinal in Engineered Rhodopsin Mimics. Chemistry - A European Journal 2016, 22: 8254-8261. PMID: 27120137, DOI: 10.1002/chem.201505126.Peer-Reviewed Original ResearchConceptsExcited state energy levelsQuantum chemical calculationsStructure of chromophoresElectronic structure of chromophoresAmount of charge transferState energy levelsIn silico mutationsChemical calculationsSchiff-baseCharge transferRhodopsin mimicAbsorption shiftElectronic structureRational designElectrostatic effectsEnergy levelsVisible spectrumChromophoreAbsorption propertiesInfrared regionNative chemicalHuman cellular retinol-binding proteinB-iononeBiological environmentHCRBPII
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